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Combining short-circuited t-HP and half-reactions e-HP in one continuous flow reactor

Subject Area Chemical and Thermal Process Engineering
Term since 2024
Project identifier Deutsche Forschungsgemeinschaft (DFG) - Project number 525028514
 
The hypothesis that the t-HP catalyst acts as a "short-circuited" electrochemical cell represents a compelling paradigm shift. Nevertheless, a thorough study considering this notion is challenging owing to the inherent transport limitations of the reactions and the fact that e-HP is typically done at atmospheric pressure while t-HP is greatly accelerated at high pressure. Consequently, comparative analyses of t-HP and e-HP have so far, been relegated to separate, specialized reactors. As part of the Research Unit HyPerCat, TP2-Dittmeyer aims to bridge this gap by developing a multifaceted experimental platform capable of seamlessly transitioning between t-HP and e-HP modalities. These "LEGO-Like" are continuous flow reactors that enable the investigation of both reaction systems under controlled thermodynamic and flow conditions. Our goal is thus, to attain a profound phenomenological understanding that will be the basis of the rational design of reaction systems for both t-HP and e-HP. Three convergent elements will be part of TP2: 1) Integrated fabrication of micro-structured elements through additive manufacturing, 2) Precision technical coating of catalysts in the resulting devices and 3) Experimentally validated CFD modelling of the reaction conditions and product evolution.
DFG Programme Research Units
 
 

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