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Coupled dynamics of polarization and magnetization in ferroelectric-magnetic layers

Subject Area Theoretical Condensed Matter Physics
Term from 2011 to 2014
Project identifier Deutsche Forschungsgemeinschaft (DFG) - Project number 188443797
 
Final Report Year 2015

Final Report Abstract

The project is focused on novel materials - two phase multiferroics, exhibiting coupled ferroelectric and ferromagnetic orders. Aiming at developing a numerical method to couple the magnetization dynamics based on the Landau-Lifhitz-Gilbert equation with the polarization dynamics using the Landau-Khalatnikov equation as well as using Monte-Carlo methods, peculiarities of the switching behavior of ferroelectric and ferromagnetic orders were demonstrated depending on the type of the coupling between the orders. In particular, using as a prototype structure an interface of Fe/BaTiO3, where a strong charge-mediated magneto electric coupling has been evidenced, it was shown that though the subsystems are coupled, the ferroelectric subsystem responses to an external time-dependent electric field on the time scale of several picoseconds, whereas the magnetic subsystem requires up to several hundreds of picoseconds to be fully switched. The effect of the strain-mediated coupling was separately inspected for the same interface, where an externally applied time-dependent electric field caused an interfacial stress of the ferroelectric and resulted in a modified anisotropy of the ferromagnet modifying thus the magnetization. Additionally, within the present calculations the effect of ferromagnetic resonance for Fe/BaTiO3-interface was demonstrated to reveal the strength and the symmetry of the magnetoelectric coupling, which was corroborated in a subsequent experiment. The proposed methods clarified the role of thermal fluctuations in two-phase multiferroics and rendered possible a demonstration of multiferroic systems for signal handling processes.

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